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| 1 | 船只排放物对欧洲空气质量及酸性沉降造成的影响显示文摘一个名为'STOCHEM'的三维拉氏化学传输模型被用于描述2000年气候条件下国际海运活动产生的SO_2、NO_x、VOCs和CO排放造成的欧洲大西洋沿岸区域性酸性沉降和臭氧空气质量影响的状况。该模型得出的从西南海域到不列颠群岛和布列塔尼水域国际海运活动产生的硫沉降总量高达200mg/m^2·a。夏季国际海运活动对表层臭氧浓度的影响在爱尔兰、布列塔尼和葡萄牙高达约6ppb。在欧洲,海运活动产生的排放物是一种对酸性沉降和臭氧空气质量造成影响的外部因素,并且如果要在将来达到严格的沉降及空气质量目标,就需要采取一系列控制措施。 | Richard G.Derwent David S.Stevenson Ruth M.Doherty William J.Collins Michael G.Sanderson Colin E.Johnson Janusz Cofala Reinhard Mechler Markus Amann Frank J.Dentener 许天虎 | 2005 | AMBIO-人类环境杂志2005,34,1: | 2 |
| 2 | Historyof knee injuries and knee osteoarthritis:a meta-analysis of observational studies显示文摘 | S.G.Muthuri D.F.McWilliams M.Doherty | | 0,,: | 1 |
| 3 | Underlying solvent-based factors that influence permanent porosity in porous liquids显示文摘Porous liquids(PLs)offer the potential to combine the ready handling and mature industry status of liquid absorbents,with the high permanent porosity of metal organic frameworks.To be functional,these nanocomposites need to satisfy a number of performance parameters,such as stability and viscosity of the porogen-solvent combination,avoiding solvent penetration into metal organic framework(MOF)pores,suitable capacities,and kinetics for gas sorption.In this work,we systematically investigate the component materials to elucidate the parametric space where stable photoluminescence(PL)can be generated.In this situation,deeper conclusions were able to be drawn with regard to the influence of hydrophobicity/philicity on the properties of the resulting nanocomposites.Zeolitic imidazolate frameworks(ZIFs)were combined with a range of solvents varying in steric bulk,to deliver CO_(2)sorption capacities as high as 4.2 mmol·g^(-1)at 10 bar.These findings may have broader implications for future investigations of this tantalising field of nanocomposites. | Hamidreza Mahdavi Huacheng Zhang Lauren K.Macreadie Cara M.Doherty Durga Acharya Stefan J.DSmith Xavier Mulet Matthew R.Hill | 2022 | Nano Research2022,15,4: | 1 |
| 4 | Investigation of the effects of ion and water interaction on structure and chemistry of silicalite MFI type zeolite for its potential use as a seawater desalination membrane显示文摘 | Bo Zhu Linda Zou Cara M.Doherty | | 0,,: | 1 |
| 5 | Effects of complementary therapies on clinical outcomes in patients being treated with radiation therapy for prostate cancer显示文摘 | ClairBeard William B.Stason QianWang JudithManola ElizabethDean‐Clower Jeffery A.Dusek SusanDeCristofaro AnnWebster Anne M.Doherty‐Gilman David S.Rosenthal HerbertBenson | 2010 | Cancer2010,,: | 1 |
| 6 | Porous solid inspired hyper-crosslinked polymer liquids with highly efficient regeneration for gas purification显示文摘Separation media that combine the desired material properties within a single material for a given process remain an ongoing challenge for the gas separations in industry.Process integration of porous solid adsorbents is difficult due to their limited volumetric capacity,whereas issues of volatility and high regeneration temperatures exist for liquid amines and physical solvents.Herein,we report a family of polymer liquids inspired by hyper-crosslinked polymers(HCPs),a class of highly swellable network polymers.Compared with a chemically similar porous solid,the HCP-liquids demonstrate good volumetric capacity and improved selectivity of carbon dioxide over methane.Uptake appears to be enhanced by intramolecular swelling of the HCP-liquids at elevated pressures,while guests are strongly rejected from the HCP-liquids at slightly elevated temperatures,leading to highly efficient regeneration.Heat of adsorption and specific heat capacity of the HCP-liquids are also low,further suggesting favourable process thermodynamics.Additionally being easily prepared at scale,the presented HCP-liquids represent a promising step towards a material with the requisite properties to replace conventional scrubbing solvents to drastically reduce the footprint and energy needs of gas separations. | Stefan J.D.Smith Colin D.Wood Paul H.M.Feron Hamidreza Mahdavi Roger J.Mulder Cara M.Doherty Matthew R.Hill Xavier Mulet | 2022 | Science China Materials2022,65,7: | 0 |
| 7 | 臭氧浓度响应函数与日死亡率显示文摘[背景]短期臭氧暴露与日死亡率增加相关。浓度-反应关系的形状对于估算公众健康影响至关重要,特别是假设存在阈值时。[目的]研究1993—2006年间,英国5个城市及5个乡村地区每日臭氧暴露浓度与死亡率之间的浓度-反应关系。[方法]采用泊松回归,控制季节性、温度和流感等变量,分析每日最大8h臭氧浓度与每日全死因死亡率之间的相关性,分别为全年及特定季节假设了线性、线性阈值和样条模型。作者还检测了灵敏度以及替代温度指标,前者用以调整对颗粒物的测定(仅限市区)。[结果]在所有年份的分析中,在伦敦发现臭氧与全死因死亡率的浓度-反应关系中存在明确的阈值,为65μg/m(395%CI:58~83);但是,在其他城市或乡村地区存在阈值的证据却很少。综合线性效应估计城市和乡村地区的全死因死亡率具有可比性:臭氧浓度每增加10μg/m3,全死因死亡率分别增加0.48%(95%CI:0.35~0.60)和0.58%(95%CI:0.36~0.81)。季节性分析表明,夏季的月份中在城市和乡村地区都存在臭氧影响的阈值。[结论]应该采用阈值和非阈值模型评价整个环境范围内臭氧对健康的影响,并且根据季节进行分层。在伦敦存在阈值效应,但在其他研究区域却未发现,这一点需要进一步研究探讨。乡村地区臭氧暴露对公众健康的影响不容忽视。 | Richard W.Atkinson Dahai Yu Ben G.Armstrong Sam Pattenden Paul Wilkinson Ruth M.Doherty Mathew R.Heal H.Ross Anderson | 2013 | 环境与职业医学2013,30,1: | 0 |