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| 1 | Highly Selective Biomimetic Flexible Tactile Sensor for Neuroprosthetics显示文摘Biomimetic flexible tactile sensors endow prosthetics with the ability to manipulate objects,similar to human hands.However,it is still a great challenge to selectively respond to static and sliding friction forces,which is crucial tactile information relevant to the perception of weight and slippage during grasps.Here,inspired by the structure of fingerprints and the selective response of Ruffini endings to friction forces,we developed a biomimetic flexible capacitive sensor to selectively detect static and sliding friction forces.The sensor is designed as a novel plane-parallel capacitor,in which silver nanowire-3D polydimethylsiloxane(PDMS)electrodes are placed in a spiral configuration and set perpendicular to the substrate.Silver nanowires are uniformly distributed on the surfaces of 3D polydimethylsiloxane microcolumns,and silicon rubber(Ecoflex^(■))acts as the dielectric material.The capacitance of the sensor remains nearly constant under different applied normal forces but increases with the static friction force and decreases when sliding occurs.Furthermore,aiming at the slippage perception of neuroprosthetics,a custom-designed signal encoding circuit was designed to transform the capacitance signal into a bionic pulsed signal modulated by the applied sliding friction force.Test results demonstrate the great potential of the novel biomimetic flexible sensors with directional and dynamic sensitivity of haptic force for smart neuroprosthetics. | Yue Li Zhiguang Cao Tie Li Fuqin Sun Yuanyuan Bai Qifeng Lu Shuqi Wang Xianqing Yang Manzhao Hao Ning Lan Ting Zhang | 2020 | Research2020，，1： | 4 |
| 2 | Biological receptor-inspired flexible artificial synapse based on ionic dynamics显示文摘The memristor has been regarded as a promising candidate for constructing a neuromorphic computing platform that is capable of confronting the bottleneck of the traditional von Neumann architecture.Here,inspired by the working mechanism of the G-protein-linked receptor of biological cells,a novel double-layer memristive device with reduced graphene oxide(rGO)nanosheets covered by chitosan(an ionic conductive polymer)as the channel material is constructed.The protons in chitosan and the functional groups in rGO nanosheets imitate the functions of the ligands and receptors of biological cells,respectively.Smooth changes in the response current depending on the historical applied voltages are observed,offering a promising pathway toward biorealistic synaptic emulation.The memristive behavior is mainly a result of the interaction between protons provided by chitosan and the defects and functional groups in the rGO nanosheets.The channel current is due to the hopping of protons through functional groups and is limited by the traps in the rGO nanosheets.The transition from short-term to long-term potentiation is achieved,and learning-forgetting behaviors of the memristor mimicking those of the human brain are demonstrated.Overall,the bioinspired memristor-type artificial synaptic device shows great potential in neuromorphic networks. | Qifeng Lu Fuqin Sun Lin Liu Lianhui Li Yingyi Wang Mingming Hao Zihao Wang Shuqi Wang Ting Zhang | 2020 | Microsystems & Nanoengineering2020，6，1： | 2 |
| 3 | Bio-inspired flexible artificial synapses for pain perception and nerve injuries显示文摘Imitation of the perception system of living creatures is of great importance for the construction of artificial nerves and intelligent human-machine interfaces.However,a prominent challenge is to emulate the functions of the biological synapse,which is the basic building block of the neural system.Here,inspired by the pain perception mechanism of the living creatures,a flexible double-layer memristor was constructed,with 90%semiconducting single-wall carbon nanotubes(s-SWCNTs)covered by LiClO4 doped polyoxyethylene oxide(PEO:LiClO4)as the channel materials.The carriers(protons and Li+)from PEO:LiClO4 imitated the functions of Na+and K+in biological systems.A potentiation of the post-synaptic signal was observed with mild stimuli,while the post-synaptic signal was inhibited with severe stimuli with a pulse voltage larger than 1.4 V in this research.These behaviors resemble the sensation of pain,neuroprotection,and possible injuries to the neural system.To explore the underlying mechanism of the phenomenon,the fourier-transform infrared spectroscopy(FTIR),X-ray photoelectron spectroscopy(XPS),Raman spectrum,and current(IV)sweep were carried out.It was inferred that the observed results are attributable to the interaction between carriers in PEO:LiClO4 and functional groups and defects in the s-SWCNTs.The enhanced channel current results from the fulfillment of the traps by the carriers,and the suppression of the current is due to the intercalation of Li+in the s-SWCNTs.This flexible artificial synapse opens a new avenue for the construction of biocompatible electronic devices towards artificial intelligence systems. | Qifeng Lu Fuqin Sun Lin Liu Lianhui Li Mingming Hao Zihao Wang Ting Zhang | 2020 | npj Flexible Electronics2020，4，1： | 1 |
| 4 | “Top-down” and “bottom-up” strategies for wafer-scaled miniaturized gas sensors design and fabrication显示文摘Manufacture of large-scale patterned nanomaterials via top-down techniques,such as printing and slurry coating,have been used for fabrication of miniaturized gas sensors.However,the reproducibility and uniformity of the sensors in wafer-scale fabrication are still a challenge.In this work,a“top-down”and“bottom-up”combined strategy was proposed to manufacture wafer-scaled miniaturized gas sensors with high-throughput by in-situ growth of Ni(OH)2 nanowalls at specific locations.First,the micro-hotplate based sensor chips were fabricated on a two-inch(2″)silicon wafer by micro-electro-mechanical-system(MEMS)fabrication techniques(“top-down”strategy).Then a template-guided controllable de-wetting method was used to assemble a porous thermoplastic elastomer(TPE)thin film with uniform micro-sized holes(relative standard deviation(RSD)of the size of micro-holes<3.5%,n>300),which serves as the patterned mask for in-situ growing Ni(OH)2 nanowalls at the micro-hole areas(“bottom-up”strategy).The obtained gas microsensors based on this strategy showed great reproducibility of electric properties(RSD<0.8%,n=8)and sensing response toward real-time H _(2)S detection(RSD<3.5%,n=8). | Lin Liu Yingyi Wang Fuqin Sun Yanbing Dai Shuqi Wang Yuanyuan Bai Lianhui Li Tie Li Ting Zhang Sujie Qin | 2020 | Microsystems & Nanoengineering2020，6，1： | 1 |
| 5 | One-step synthesis of biomass derived O, N-codoped hierarchical porous carbon with high surface area for supercapacitors显示文摘We report a convenient method to synthesize O,N-codoped hierarchical porous carbon by one-step carbonization of the mixture of KHCO3,urea and alginic acid.Benefiting from KHCO3 and urea syne rgistic effect,the obtained O,N-codoped hierarchical porous carbon(NPC-700) material has a well-developed interconnected porous framework with ultrahigh specific surface area(2846 m2/g) and massive heteroatoms functional groups.Consequence,such porous carbon displays high specific capacitance(324 F/g at 1 A/g),excellent rate performance(212 F/g at 30 A/g) and good electrochemical stabilization in 6 mol/L KOH solution.More importantly,the assembled NPC-700//NPC-700 symmetrical supercapacitor can achieve a high energy density of 18.8 Wh/kg and good electrochemical stabilization in 1 mol/L Na2SO4 solution.This process opens up a new way to design heteroatoms-doped hierarchical porous carbon derived from biomass materials for supercapacitors. | Shuxian Sun Fuqin Han Xiaoliang Wu Zhuangjun Fan | 2020 | Chinese Chemical Letters2020，31，9： | 1 |
| 6 | Turing pattern of the Oregonator model 显示文摘 | Peng Rui Sun Fuqin | 2010 | Nonlinear Analysis2010，72，5： | 1 |
| 7 | Asymptotically Self-Similar Global Solutions for a Higher-Order Semilinear Parabolic System显示文摘 | SUN Fuqin LI Fan JIA Xiuqing | 2009 | Journal of Partial Differential Equations2009，22，3： | 1 |
| 8 | Stretchable,self-healing,transient macromolecular elastomeric gel for wearable electronics显示文摘Flexible and stretchable electronics are emerging in mainstream technologies and represent promising directions for future lifestyles.Multifunctional stretchable materials with a self-healing ability to resist mechanical damage are highly desirable but remain challenging to create.Here,we report a stretchable macromolecular elastomeric gel with the unique abilities of not only self-healing but also transient properties at room temperature.By inserting small molecule glycerol into hydroxyethylcellulose(HEC),forming a glycerol/hydroxyethylcellulose(GHEC)macromolecular elastomeric gel,dynamic hydrogen bonds occur between the HEC chain and the guest small glycerol molecules,which endows the GHEC with an excellent stretchability(304%)and a self-healing ability under ambient conditions.Additionally,the GHEC elastomeric gel is completely water-soluble,and its degradation rate can be tuned by adjusting the HEC molecular weight and the ratio of the HEC to glycerol.We demonstrate several flexible and stretchable electronics devices,such as self-healing conductors,transient transistors,and electronic skins for robots based on the GHEC elastomeric gel to illustrate its multiple functions. | Mingming Hao Lianhui Li Shuqi Wang Fuqin Sun Yuanyuan Bai Zhiguang Cao Chunyan Qu Ting Zhang | 2019 | Microsystems & Nanoengineering2019，5，1： | 1 |
| 9 | Global dynamics of a predator-prey model incorporating a constant prey refuge显示文摘 | Xiaolei Yu Fuqin Sun | 2013 | Electronic Journal of Differential Equations2013，4，： | 1 |
| 10 | A hybrid flexible gas sensory system with perceptual learning显示文摘Imbuing artificial sensory system with intelligence of the biological counterpart is limited by challenges in emulating perceptual learning ability at the device level.In biological systems,stimuli from the surrounding environment are detected,transmitted,and processed by receptor,afferent nerve,and brain,respectively.This process allows the living creatures to identify the potential hazards and improve their adaptability in various environments.Here,inspired by the biological olfaction system,a gas sensory system with perceptual learning is developed.As a proof-of-concept,H2S gas with various concentrations is used as the stimulation and the stimuli will be converted to pulse-like physiological signals in the designed system,which consists of a gas sensor,a flexible oscillator,and a memristor-type artificial synapse.Furthermore,the learning ability is implemented using a supervised learning method based on k-nearest neighbors(KNN)algorithm.The recognition accuracy can be enhanced by repeating training,illustrating a great potential to be used as the neuromorphic sensory system with a learning ability for the applications in robotics. | Qifeng Lu Fuqin Sun Yanbing Dai Yingyi Wang Lin Liu Zihao Wang Shuqi Wang Ting Zhang | 2022 | Nano Research2022，15，1： | 0 |
| 11 | Stable epidermal electronic device with strain isolation induced by in situ Joule heating显示文摘Epidermal electronics play increasingly important roles in human-machine intetfaces.However,their efficient fabrication while maintaining device stability and reliability remains an unresolved challenge.Here,a facile in situ Joule heating method is proposed for fabricating stable epidermal electronics on a polyvinyl alcohol(PVA)substrate.Benefiting from the precise control of heating locations,the crystallization and enhanced rigidity of PVA are restricted to desired areas,leading to strain isolation of the active regions.As a result,the electronic device can be conformably attached to skin while showing negligible degradation in device performance during deformation.Based on this method,a flexible surface electromyography(sEMG)sensor with outstanding stability and highly comfortable wearability is demonstrated,showing high accuracy(91.83%)for human hand gesture recognition.These results imply that the fabrication method proposed in this research is a facile and reliable approach for the fabrication of epidermal electronics. | Zihao Wang Qifeng Lu Yizhang Xia Simin Feng Yixiang Shi Shuqi Wang Xianqing Yang Yangyong Zhao Fuqin Sun Tie Li Ting Zhang | 2021 | Microsystems & Nanoengineering2021，7，4： | 0 |
| 12 | Multifunctional biomimetic tactile system via a stick-slip sensing strategy for human–machine interactions显示文摘A tactile sensor system enables natural interaction between humans and machines;this interaction is crucial for dexterous robotic hands,interactive entertainment,and other smart scenarios.However,the lack of sliding friction detection significantly limits the accuracy and scope of interactions due to the absence of sophisticated information,such as slippage,material and roughness of held objects.Here,inspired by the stick-slip phenomena in the sliding process,we have developed a multifunctional biomimetic tactile system based on the stick-slip sensing strategy,which is a universal method to detect slippage and estimate the surface properties of objects by sliding.This system consists of a flexible fingertip-inspired tactile sensor,a read-out circuit and a machinelearning module.Based on the stick-slip sensing strategy,our system was endowed with high recognition rates for slippage detection(100.0%),material classification(93.3%)and roughness discrimination(92.8%).Moreover,robotic hand manipulation,interactive games and object classification are demonstrated with this multifunctional system for comprehensive and promising human-machine interactions. | Yue Li Manjun Zhao Yadong Yan Luanxi He Yingyi Wang Zuoping Xiong Shuqi Wang Yuanyuan Bai Fuqin Sun Qifeng Lu Yu Wang Tie Li Ting Zhang | 2022 | npj Flexible Electronics2022，6，1： | 0 |
| 13 | An artificial neuromorphic somatosensory system with spatio-temporal tactile perception and feedback functions显示文摘The advancement in flexible electronics and neuromorphic electronics has opened up opportunities to construct artificial perception systems to emulate biological functions which are of great importance for intelligent robotics and human-machine interactions.However,artificial systems that can mimic the somatosensory feedback functions have not been demonstrated yet despite the great achievement in this area.In this work,inspired by human somatosensory feedback pathways,an artificial somatosensory system with both perception and feedback functions was designed and constructed by integrating the flexible tactile sensors,synaptic transistor,artificial muscle,and the coupling circuit.Also,benefiting from the synaptic characteristics of the designed artificial synapse,the system shows spatio-temporal information-processing ability,which can further enhance the efficiency of the system.This research outcome has a potential contribution to the development of sensor technology from signal sensing to perception and cognition,which can provide a special paradigm for the next generation of bionic tactile perception systems towards e-skin,neurorobotics,and advanced bio-robots. | Fuqin Sun Qifeng Lu Mingming Hao Yue Wu Yue Li Lin Liu Lianhui Li Yingyi Wang Ting Zhang | 2022 | npj Flexible Electronics2022，6，1： | 0 |
| 14 | Biological Tissue-Inspired Ultrasoft,Ultrathin,and Mechanically Enhanced Microfiber Composite Hydrogel for Flexible Bioelectronics显示文摘Hydrogels offer tissue-like softness,stretchability,fracture toughness,ionic conductivity,and compatibility with biological tissues,which make them promising candidates for fabricating flexible bioelectronics.A soft hydrogel film offers an ideal interface to directly bridge thin-film electronics with the soft tissues.However,it remains difficult to fabricate a soft hydrogel film with an ultrathin configuration and excellent mechanical strength.Here we report a biological tissue-inspired ultrasoft microfiber composite ultrathin(<5μm)hydrogel film,which is currently the thinnest hydrogel film as far as we know.The embedded microfibers endow the composite hydrogel with prominent mechanical strength(tensile stress~6 MPa)and anti-tearing property.Moreover,our microfiber composite hydrogel offers the capability of tunable mechanical properties in a broad range,allowing for matching the modulus of most biological tissues and organs.The incorporation of glycerol and salt ions imparts the microfiber composite hydrogel with high ionic conductivity and prominent anti-dehydration behavior.Such microfiber composite hydrogels are promising for constructing attaching-type flexible bioelectronics to monitor biosignals. | Qiang Gao Fuqin Sun Yue Li Lianhui Li Mengyuan Liu Shuqi Wang Yongfeng Wang Tie Li Lin Liu Simin Feng Xiaowei Wang Seema Agarwal Ting Zhang | 2023 | Nano-Micro Letters2023，15，9： | 0 |
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